Spain is a country located at the Iberia peninsula in Southwestern Europe. It is known as the "Land of Toros" by Grandpa Smurf as bullfight (toro) are one of the iconic entertainments of Spain.
In the episode "Papa Loses His Patience", the Smurfs visits there by the time crystals. In the episode, Papa Smurf loses his patience by Brainy's magic potion, and they get Papa Smurf's patience back from the bullfighter El Gargo, who gets Papa Smurf's patience accidentally.
In Lleida, Spain, a Smurfs theme park was built and has opened in 2020.